Congrats to Jinyu Zhang, Bin Lu, Zhaoliang Ge et al. for the latest publication in Org. Lett. A novel [Rh]2-catalyzed three-component reaction of readily accessible indoles, diazo compounds, and allylic compounds is developed via a relay carbene-induced C-H functionalization and allylic alkylation process, affording diverse C3-substituted indoles bearing all-carbon quaternary centers in good yields with high atom and step economy.